To develop the photoelastic experiment method for the orthotropic material under pure torsional moment is the main objective of this research. In the development of photoelastic experiment for orthotropic material under pure torsional moment, the important problems and their solutions are the same as following. In the model material for photoelastic experiment, it was found that C.F.E.C.(Copper Fiber Epoxy Composite) can be used as the model material of photoelastic experiment for orthotropic material. In the stress freezing cycle, it was assured that stress freezing cycle for epoxy can be used as the stress freezing cycle of the photoelastic experiment for orthotropic material. In the slicing method, it was found that the negative oblique slicing method can be effectively used as slicing method in 3-dimensional photoelastic experiment. In the measuring method of stress fringe values and physical properties in the high temperature, it was found that stress fringe values can be directly measured by experiment and physical properties can be directly or indirectly by equation between stress fringe values and physical properties developed by author. In the stress analysis method of orthotropic material under pure torsional moment by photoelastic experiment, it will be studied in the second paper.