This paper deals with an experimental investigation on an active vibration control of ahybrid smart structure(HSS) via an electro-rheological fluid actuator(ERFA) and a piezoelectric film actuator(PFA). Firstly, an HSS is constructed by inserting a silicone oil-based electro-rheological fluid into a hollow can- tilevered beam and perfectly bonding piezoelectric films ofn the upper and lower surfaces of the beam as an actuator and a sensor, respectively. The control scheme of the ERFA tuning stiffness and damping charac- teristics of the HSS with imposed electric fields is formulated as a function of excitation frequencies on the basis of field-dependent respnses. On the other hand, as for the control scheme of the PFA permitting control voltages to generate axial forces or bending moments for suppressing deflections of the HSS, a neuro sliding mode controller(NSC) is employed. Furthermore, an experimental implementation activating the ERFA and the PFA independently is established to carry out an active vibration control in both the transient and forced vibrations. The experimental results exhibit a superior ability of the gtbrid actuation system to tailor elastodynamic response characteristics of the HSS rather than a single class of actuator system alone.