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Metal-Insulator Transition Induced by Short Range Magnetic Ordering in Mono-layered Manganite
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  • Metal-Insulator Transition Induced by Short Range Magnetic Ordering in Mono-layered Manganite
  • Metal-Insulator Transition Induced by Short Range Magnetic Ordering in Mono-layered Manganite
저자명
Chi. E.O.,Kim. W.S.,Hong. C.S.,Hur. N.H.,Choi. Y.N.
간행물명
Bulletin of the Korean Chemical Society
권/호정보
2003년|24권 5호|pp.573-578 (6 pages)
발행정보
대한화학회
파일정보
정기간행물|ENG|
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이 논문은 한국과학기술정보연구원과 논문 연계를 통해 무료로 제공되는 원문입니다.
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기타언어초록

The structural, magnetic, and transport properties of a mono-layered manganite $La_{0.7}Sr_{1.3}MnO_{4+{delta}}$ were investigated using variable temperature neutron powder diffraction as well as magnetization and transport measurements. The compound adopts the tetragonal I4/mmm symmetry and exhibits no magnetic reflection in the temperature region of 10 K ≤ T ≤ 300 K. A weak ferromagnetic (FM) transition occurs about 130 K, which almost coincides with the onset of a metal-insulator (M-I) transition. Extra oxygen that occupies the interstitial site between the [(La,Sr)O] layers makes the spacing between the [MnO₂] layers shorten, which enhances the inter-layer coupling and eventually leads to the M-I transition. We also found negative magneto resistance (MR) below the M-I transition temperature, which can be understood on the basis of the percolative transport via FM metallic domains in the antiferromagnetic (AFM) insulating matrix.