A measured frequency response function can be represented as a ratio of two polynomials. A curve-fitting of frequency responses with Legendre polynomialis suggested in the paper. And the suggested curve-fitting algorithm is based on the least-square error method. Since the Legendre polynomials satisfy the orthogonality condition, the curve-fitting with the polynomials results to more reliable curve-fitting than ordinary polynomial method. Though the proposed curve-fitting with Legendre polynomials cannot cover all frequency range of interest, example shows that the suggested method is quite applicable in a limited frequency band.