NMR over 1 GHz (23.5 T) level has difficulties in design and fabrication with only low temperature superconducting (LTS) wire because of its material characteristics such as the decay of critical current under the magnetic field. Because High temperature superconducting (HTS) tape has a good performance under the extremely high magnetic field, it has been developed for high-field magnet over 23.5 T. In this paper, the LTS magnet was made for applying magnetic fields externally and the HTS coil was designed and fabricated. The electromagnetic field analysis has been done with respect to the structure and the operating current of the LTS and HTS coil. Considering to the field homogeneity and the center field, the design parameters which is suitable for the HTS coil were found. The HTS insert coil was impregnated with epoxy resin in order to prevent the movement of winding during energizing the magnet. The hybrid magnet (LTS/HTS) magnet was fabricated and tested based on the design parameters. The experimental result shows that the LTS background magnet and the HTS insert coil can be operated stable beyond 220 A and 210 A. The final value 4.32 T at the center was acquired.