In order to capture the fast crack propagation in an unmanipulated concrete fracture test, we employed mechanoluminascent(ML) material, which emits visible light when stressed, as a crack visualization tool. Three-point bending fracture test setup, a paint type ML material and a high speed camera were used to capture the images of fast moving cracks. The maximum size of coarse aggregates of concrete was used as an experimental parameter. The crack images, loading, and crack mouth opening displacement were successfully recorded as a function of time elapsed. From the test results, several interesting cracking behavior in the unmanipulated fracture test was observed in such that (1) the crack moves fast while the load is slowly decreased after the maximum loading, and (2) the crack in concrete with larger coarse aggregates moves faster than the others.